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How "quantum" is the exciton dynamics in the Fenna-Matthews-Olson complex?.
(arXiv:1104.2031v1 [cond-mat.mes-hall])
Authors: Peter Nalbach, Daniel Braun, Michael Thorwart
We present numerically exact results for the quantum coherent energy transfer
in the Fenna-Matthews-Olson molecular aggregate under realistic physiological
conditions, including also vibrational fluctuations of the protein and the
pigments. We find that although the coherence times are to some extent reduced
as compared to the often assumed Ohmic fluctuation spectrum, the exciton
dynamics is far from being a classical hoping process. We quantify the
"quantumness" of the energy transfer as distance of the density matrix to the
classical pointer states for the energy current operator.
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